He’s really good as a villain
Just pure evil
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He’s insane.
Does Loki still count as a villain? If yes, I choose him 
But for many people he’s “just” an anti-hero now, not a real villain
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If he counts as one to you then I say yes, as it’s based on your opinion, right?
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As in villain I love to hate the most, Umbridge from Harry Potter for sure. For actually most likeable villain, I’m not too sure honestly…
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I hate her so much.
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I can’t stand her, I hate her so much more than Voldemort, she’s like the definition of evil in my opinion.
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Akutagawa Ryunosuke from Bungo Stray Dogs. SOMEONE HUG HIM.
I gotta agree with these
Also Light from death note, probably one of the most interesting villains so far
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Potato chips.
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Iconic 
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My favorite villain from Peter Pan is Captain Hook, because he’s a pirate and I find his backstory interesting.